| Summary: | The current research investigates the impact of magnetite (Fe3O4) nanoparticles (3–12 wt%) on the properties of rubbery polymer nanocomposites fabricated via melt blending method. The tensile and impact properties were improved at an optimal 6 wt% Fe3O4, revealing a good interfacial interaction. Fe3O4 enhanced the thermal stability, as evidenced by the increased integral procedure decomposition temperature up to 26 %. Fe3O4 increased residual and saturated magnetization the most at 6 wt% loading. The gamma-ray shielding properties were explored with energy ranging from 0.2835 to 2.506 MeV, and effectively at low energies. Increased Fe3O4 content correlated positively with linear attenuation coefficient (LAC), enhancing radiation shielding but reducing neutron shielding. At 0.2835 MeV, the LAC values increased up to 0.12431 cm−1 for 12 wt% Fe3O4, while the fast neutron removal cross-section values decreased from 0.10427 cm−1 to 0.08548 cm−1. These findings highlight the multifunctional potential of Fe3O4-incorporated nanocomposites in radiation shielding applications. © 2024 Elsevier Ltd
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